Femtosecond nonlinear refraction of 2D semi-metallic redox exfoliated ZrTe2at 800 nm

dc.contributor.authorMaldonado M.
dc.contributor.authorDa Silva Neto M.L.
dc.contributor.authorVianna P.G.
dc.contributor.authorRibeiro H.B.
dc.contributor.authorDe Araujo C.B.
dc.contributor.authorMatos C.J.S.D.
dc.contributor.authorSeixas L.
dc.contributor.authorJawaid A.M.
dc.contributor.authorBusch R.
dc.contributor.authorRitter A.J.
dc.contributor.authorVaia R.A.
dc.contributor.authorGomes A.S.L.
dc.date.accessioned2024-03-12T19:21:43Z
dc.date.available2024-03-12T19:21:43Z
dc.date.issued2021
dc.description.abstract© 2021 Author(s).Zirconium telluride, a transition metal dichalcogenide, was synthesized by a redox exfoliated method to obtain a 2D monolayer semi-metal. After being characterized for compositional and optical analysis, its third-order nonlinear optical (NLO) properties were studied by the Z-scan technique in the femtosecond (100 fs) regime at 800 nm. Interestingly, in this spectro-temporal regime and in the intensity range exploited, the only third-order NLO effect observed was nonlinear refraction, giving rise to a positive value of the nonlinear refractive index coefficient, n2 = +(4.2 ± 0.3) × 10-16 cm2/W. Based on the calculated band structure and the excitation photon energies employed, the physical origin of the refractive nonlinearity is discussed.
dc.description.issuenumber1
dc.description.volume118
dc.identifier.doi10.1063/5.0031649
dc.identifier.issn0003-6951
dc.identifier.urihttps://dspace.mackenzie.br/handle/10899/34725
dc.relation.ispartofApplied Physics Letters
dc.rightsAcesso Restrito
dc.titleFemtosecond nonlinear refraction of 2D semi-metallic redox exfoliated ZrTe2at 800 nm
dc.typeArtigo
local.scopus.citations13
local.scopus.eid2-s2.0-85099238418
local.scopus.subjectNon-linear refraction
local.scopus.subjectNonlinear refractive index coefficient
local.scopus.subjectOptical analysis
local.scopus.subjectRefractive non-linearity
local.scopus.subjectTemporal regimes
local.scopus.subjectThird-order nonlinear optical
local.scopus.subjectTransition metal dichalcogenides
local.scopus.subjectZ-scan technique
local.scopus.updated2024-11-01
local.scopus.urlhttps://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=85099238418&origin=inward
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